(Not quite sure of the format of your .srt's, but...)
Everything.
Search for (I'm going to use .7z with .exe before it as an example, but substitute .srt with .en for your case...):
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ext:exe.7z ext:7z
That says to find files with a .7z extension AND files with a .exe.7z "extension".
(That's actually the same as leaving out the latter part, ext:7z.)
But you can also:
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!ext:exe.7z ext:7z
And that says to find files with a .7z extension AND NOT those files that end in .exe.7z.
So, the first search finds:
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123VIEW.EXE.7z
2GIF.EXE.7z
7z1512.exe.7z
7z1604.exe.7z
7z1805.exe.7z
ACD_CFG.EXE.7z
AVIEWNC4.EXE.7z
DBVIEW.EXE.7z
And the second search finds:
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BASIS.TEMP.7z
curl-7.57.0-win32-mingw.7z
ffmpeg-2.1-win32-shared (avcodec-55.dll).7z
FhGaacenc_3507.7z
That is .7z files without .exe.7z.
Do similar with your .srt, so search for:
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!ext:en.srt ext:srt
(Adjust as the case may be on your end.)
Should find:
14 Degrees - A Paranormal Documentary.srt
But not:
AMD Heatsink Removal & Re-Use - section4-high.en.srt
Anyhow, once the files are found (which should be all .srt without .en), drag them from Everything into BRU (it may take a couple drags as BRU is quirky with drags) & rename those files to add the .en in there.